For my pose, I'm thinking of a simple standing position with the arms down and closed fists, with the shoulder-mounted anti-personnel weapons out, to reenact the scene where he just calmly stands there and takes out all the terrorists holding the civilians hostage. That was my favorite scene in the film I think.
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That was probably my favorite moment with the Mark III armor (shooting the tank is a close second), but as a pose, it's too much like a standard museum pose for me. Without the other parts of the scene (i.e., terrorists and civilians), it's just him standing upright in his armor. As LexiKon posted, I may start with a Reindeer Games-type pose with the shoulder guns, repulsors, and forearm missile out, then tweak it from there. I also have a Cap figure, so there will be inevitable attempts at a Civil War-esque diorama.